Linear and nonlinear refractive index changes in monolayer MoSe2

Tran Ngoc Bich1, Nguyen Ngoc Hieu2,3, Ta Thi Tho4, Le Thi Ngoc Tu5, Huynh Vinh Phuc5,
1 Physics Department, University of Education, Hue University, Vietnam
2 Institute of Research and Development, Duy Tan University, Vietnam
3 Faculty of Natural Sciences, Duy Tan University, Vietnam
4 Faculty of Mechanical Engineering, National University of Civil Engineering, Vietnam
5 Department of Natural Sciences Teacher Education, Dong Thap University, Vietnam

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In this work, we study the linear, the third-order nonlinear, and the total refractive index changes (RICs) caused by both intra- and inter-band transitions in monolayer MoSe2 in the presence of a magnetic field by using the compact density matrix approach. The results show that RICs display the blue-shift behavior with the increase of the magnetic field. The Zeeman fields do not affect the peak positions but reduce slightly peak intensities. Besides, the strong spin-orbit coupling in monolayer MoSe2 causes a significant difference in the peak due to spinning up and down. The RICs due to intra-band transition display only one peak in the THz range, while the inter-band spectra show a series of peaks in the near-infrared optical range, making monolayer MoSe2 be a promising candidate for novel optoelectronic applications.

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